Dunno about a full list Maurice - there's all the usuals, Godfather, Goodfellas, Long Good Friday, The Public Enemy, but what about these:
Kiss Of Death - with Victor Mature trying to go straight and Richard Widmark's debut as giggling psycho Tommy Udo. I love this film.
Brighton Rock - course they're gangsters, they're just a bit down on their luck is all
Sexy Beast - if it didn't have that opening scene with Ray Winstone putting a flannel on his dangly bits, would they have needed a different title?
City Of God - teen gangs in Rio. If you get the chance to see this on DVD, check out the accompanying documentary - it's exactly the same story, but for real
The Wire - okay so it's not a film, but it's pretty flipping brilliant depiction of modern gangsters in Baltimore